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First off, I would like to thank Sphax for creating something to make PureBDCraft more beautiful and success than it already is. Now, I would like the items and blocks to come in 512x resolution and lower. I don't know how Cubik works, or if it's even possible. And I also do not know if you can just downsize the resolution in Cubik, or if you need to create the model over again.
Now here are some ideas for more 3D Blocks and Items.
BLOCKS
Trees - Possibly make the logs round like you did with the cactus.
Sea Lanterns - Make the dark edges of the block stick out a bit more.
Vines
Flowers (All of them)
ITEMS
Redstone - When placed, 3D redstone would be awesome
Armour (Including Horse)
Arrow - If it's not 3D already.
Clock - Make the sides of it 3D so it adds some depth.
Thank you for reading this! Have a nice day!